Dergi makalesi Açık Erişim
Coburger, Peter; Kahraman, Gizem; Straube, Axel; Hey-Hawkins, Evamarie
<?xml version='1.0' encoding='UTF-8'?> <record xmlns="http://www.loc.gov/MARC21/slim"> <leader>00000nam##2200000uu#4500</leader> <datafield tag="245" ind1=" " ind2=" "> <subfield code="a">Rhodium(i) complexes with carborane-substituted P,N ligands: investigations of electronic structure and dynamic behaviour</subfield> </datafield> <datafield tag="909" ind1="C" ind2="4"> <subfield code="p">DALTON TRANSACTIONS</subfield> <subfield code="v">48</subfield> <subfield code="n">26</subfield> <subfield code="c">9625-9630</subfield> </datafield> <controlfield tag="001">69587</controlfield> <datafield tag="980" ind1=" " ind2=" "> <subfield code="a">user-tubitak-destekli-proje-yayinlari</subfield> </datafield> <datafield tag="520" ind1=" " ind2=" "> <subfield code="a">Two distorted square-planar Rh-I complexes (1 and 2) were obtained from [{RhCl(eta(4)-cod)}(2)] and the respective P,N ligands. The metal-ligand interaction was probed with density functional theory (DFT) and ab initio (CASSCF-NEVPT2) calculations. NMR spectroscopy proved dynamic binding behaviour of the ligands in solution. The tetradenticity of the ligands also affects the electrochemical behaviour of complexes 1 and 2 significantly. Finally, preliminary catalytic studies, namely the dehydrocoupling of dimethylamine-borane, are presented.</subfield> </datafield> <datafield tag="650" ind1="1" ind2="7"> <subfield code="2">opendefinition.org</subfield> <subfield code="a">cc-by</subfield> </datafield> <datafield tag="700" ind1=" " ind2=" "> <subfield code="a">Kahraman, Gizem</subfield> </datafield> <datafield tag="700" ind1=" " ind2=" "> <subfield code="u">Univ Leipzig, Fac Chem & Mineral, Inst Inorgan Chem, Johannisallee 29, D-04103 Leipzig, Germany</subfield> <subfield code="a">Straube, Axel</subfield> </datafield> <datafield tag="700" ind1=" " ind2=" "> <subfield code="u">Univ Leipzig, Fac Chem & Mineral, Inst Inorgan Chem, Johannisallee 29, D-04103 Leipzig, Germany</subfield> <subfield code="a">Hey-Hawkins, Evamarie</subfield> </datafield> <datafield tag="980" ind1=" " ind2=" "> <subfield code="b">article</subfield> <subfield code="a">publication</subfield> </datafield> <datafield tag="542" ind1=" " ind2=" "> <subfield code="l">open</subfield> </datafield> <datafield tag="100" ind1=" " ind2=" "> <subfield code="u">Univ Leipzig, Fac Chem & Mineral, Inst Inorgan Chem, Johannisallee 29, D-04103 Leipzig, Germany</subfield> <subfield code="a">Coburger, Peter</subfield> </datafield> <datafield tag="260" ind1=" " ind2=" "> <subfield code="c">2019-01-01</subfield> </datafield> <controlfield tag="005">20210316030411.0</controlfield> <datafield tag="909" ind1="C" ind2="O"> <subfield code="o">oai:zenodo.org:69587</subfield> <subfield code="p">user-tubitak-destekli-proje-yayinlari</subfield> </datafield> <datafield tag="856" ind1="4" ind2=" "> <subfield code="z">md5:9d0694801d293b07b07c352d2de5e3ad</subfield> <subfield code="s">228</subfield> <subfield code="u">https://aperta.ulakbim.gov.trrecord/69587/files/bib-6b5c5a6e-7f0a-444d-9d7b-d41229c6ab93.txt</subfield> </datafield> <datafield tag="540" ind1=" " ind2=" "> <subfield code="u">http://www.opendefinition.org/licenses/cc-by</subfield> <subfield code="a">Creative Commons Attribution</subfield> </datafield> <datafield tag="024" ind1=" " ind2=" "> <subfield code="a">10.1039/c9dt00628a</subfield> <subfield code="2">doi</subfield> </datafield> </record>
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