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Kahraman, Abdullah; Vishlaghi, Mahsa Barzgar; Baylam, Isinsu; Ogasawara, Hirohito; Sennaroglu, Alphan; Kaya, Sarp
<?xml version='1.0' encoding='utf-8'?> <resource xmlns:xsi="http://www.w3.org/2001/XMLSchema-instance" xmlns="http://datacite.org/schema/kernel-4" xsi:schemaLocation="http://datacite.org/schema/kernel-4 http://schema.datacite.org/meta/kernel-4.1/metadata.xsd"> <identifier identifierType="URL">https://aperta.ulakbim.gov.tr/record/8809</identifier> <creators> <creator> <creatorName>Kahraman, Abdullah</creatorName> <givenName>Abdullah</givenName> <familyName>Kahraman</familyName> </creator> <creator> <creatorName>Vishlaghi, Mahsa Barzgar</creatorName> <givenName>Mahsa Barzgar</givenName> <familyName>Vishlaghi</familyName> </creator> <creator> <creatorName>Baylam, Isinsu</creatorName> <givenName>Isinsu</givenName> <familyName>Baylam</familyName> <affiliation>Koc Univ Surface Sci & Technol Ctr KUYTAM, TR-34450 Istanbul, Turkey</affiliation> </creator> <creator> <creatorName>Ogasawara, Hirohito</creatorName> <givenName>Hirohito</givenName> <familyName>Ogasawara</familyName> <affiliation>SLAC Natl Accelerator Lab, Menlo Pk, CA 94025 USA</affiliation> </creator> <creator> <creatorName>Sennaroglu, Alphan</creatorName> <givenName>Alphan</givenName> <familyName>Sennaroglu</familyName> </creator> <creator> <creatorName>Kaya, Sarp</creatorName> <givenName>Sarp</givenName> <familyName>Kaya</familyName> </creator> </creators> <titles> <title>The Fast-Track Water Oxidation Channel On Bivo4 Opened By Nitrogen Treatment</title> </titles> <publisher>Aperta</publisher> <publicationYear>2020</publicationYear> <dates> <date dateType="Issued">2020-01-01</date> </dates> <resourceType resourceTypeGeneral="Text">Journal article</resourceType> <alternateIdentifiers> <alternateIdentifier alternateIdentifierType="url">https://aperta.ulakbim.gov.tr/record/8809</alternateIdentifier> </alternateIdentifiers> <relatedIdentifiers> <relatedIdentifier relatedIdentifierType="DOI" relationType="IsIdenticalTo">10.1021/acs.jpclett.0c02190</relatedIdentifier> </relatedIdentifiers> <rightsList> <rights rightsURI="http://www.opendefinition.org/licenses/cc-by">Creative Commons Attribution</rights> <rights rightsURI="info:eu-repo/semantics/openAccess">Open Access</rights> </rightsList> <descriptions> <description descriptionType="Abstract">BiVO4 is one of the most promising photoanode materials for water-splitting systems. Nitrogen incorporation into a BiVO4 surface overcomes the known bottleneck in its charge-transfer kinetics into the electrolyte. We explored the role of nitrogen in the surface charge recombination and charge-transfer kinetics by employing transient photocurrent spectroscopy at the time scale of surface recombination and water oxidation kinetics, transient absorption spectroscopy, and X-ray photoelectron spectroscopy. We attributed the activity enhancement mechanism to the accelerated V5+/V4+ redox process, in which incorporated nitrogen suppresses a limiting surface recombination channel by increasing the oxygen vacancies.</description> </descriptions> </resource>
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