Dergi makalesi Açık Erişim
Buyukcakir, Onur; Yuksel, Recep; Begar, Ferit; Erdogmus, Mustafa; Arsakay, Madi; Lee, Sun Hwa; Kim, Sang Ouk; Ruoff, Rodney S. S.
<?xml version='1.0' encoding='UTF-8'?> <record xmlns="http://www.loc.gov/MARC21/slim"> <leader>00000nam##2200000uu#4500</leader> <datafield tag="700" ind1=" " ind2=" "> <subfield code="a">Yuksel, Recep</subfield> <subfield code="u">Eskisehir Osmangazi Univ, Dept Chem, TR-26040 Eskisehir, Turkiye</subfield> </datafield> <datafield tag="700" ind1=" " ind2=" "> <subfield code="a">Begar, Ferit</subfield> <subfield code="u">Izmir Inst Technol, Dept Chem, TR-35430 Izmir, Turkiye</subfield> </datafield> <datafield tag="700" ind1=" " ind2=" "> <subfield code="a">Erdogmus, Mustafa</subfield> <subfield code="u">Izmir Inst Technol, Dept Chem, TR-35430 Izmir, Turkiye</subfield> </datafield> <datafield tag="700" ind1=" " ind2=" "> <subfield code="a">Arsakay, Madi</subfield> </datafield> <datafield tag="700" ind1=" " ind2=" "> <subfield code="a">Lee, Sun Hwa</subfield> <subfield code="u">Inst Basic Sci IBS, Ctr Multidimens Carbon Mat, Ulsan 44919, South Korea</subfield> </datafield> <datafield tag="700" ind1=" " ind2=" "> <subfield code="a">Kim, Sang Ouk</subfield> </datafield> <datafield tag="700" ind1=" " ind2=" "> <subfield code="a">Ruoff, Rodney S. S.</subfield> </datafield> <datafield tag="909" ind1="C" ind2="4"> <subfield code="p">ACS APPLIED ENERGY MATERIALS</subfield> <subfield code="v">6</subfield> <subfield code="n">14</subfield> <subfield code="c">9</subfield> </datafield> <datafield tag="980" ind1=" " ind2=" "> <subfield code="a">user-tubitak-destekli-proje-yayinlari</subfield> </datafield> <datafield tag="540" ind1=" " ind2=" "> <subfield code="a">Creative Commons Attribution</subfield> <subfield code="u">http://www.opendefinition.org/licenses/cc-by</subfield> </datafield> <datafield tag="024" ind1=" " ind2=" "> <subfield code="a">10.1021/acsaem.3c01163</subfield> <subfield code="2">doi</subfield> </datafield> <datafield tag="245" ind1=" " ind2=" "> <subfield code="a">Ultralong-Life Quinone-Based Porous Organic Polymer Cathode for High-Performance Aqueous Zinc-Ion Batteries</subfield> </datafield> <datafield tag="100" ind1=" " ind2=" "> <subfield code="a">Buyukcakir, Onur</subfield> <subfield code="u">Izmir Inst Technol, Dept Chem, TR-35430 Izmir, Turkiye</subfield> </datafield> <datafield tag="909" ind1="C" ind2="O"> <subfield code="o">oai:aperta.ulakbim.gov.tr:267730</subfield> <subfield code="p">user-tubitak-destekli-proje-yayinlari</subfield> </datafield> <datafield tag="650" ind1="1" ind2="7"> <subfield code="2">opendefinition.org</subfield> <subfield code="a">cc-by</subfield> </datafield> <datafield tag="260" ind1=" " ind2=" "> <subfield code="c">2023-01-01</subfield> </datafield> <datafield tag="856" ind1="4" ind2=" "> <subfield code="u">https://aperta.ulakbim.gov.trrecord/267730/files/bib-5c374aec-ef39-4fd0-bf8f-ba74dc44c653.txt</subfield> <subfield code="z">md5:3fa3c9bff8b35227beb66d1b10c9cfee</subfield> <subfield code="s">259</subfield> </datafield> <datafield tag="542" ind1=" " ind2=" "> <subfield code="l">open</subfield> </datafield> <controlfield tag="005">20240607125418.0</controlfield> <controlfield tag="001">267730</controlfield> <datafield tag="980" ind1=" " ind2=" "> <subfield code="a">publication</subfield> <subfield code="b">article</subfield> </datafield> <datafield tag="520" ind1=" " ind2=" "> <subfield code="a"><p>We synthesized and studied a redox-active quinone-basedporousorganic polymer (rPOP) and found ultralong cycle life: it is a promisingorganic cathode for aqueous zinc-ion batteries (ZIBs). It has highphysicochemical stability and enhanced intrinsic conductivity fromits fused-aromatic conjugated skeleton. rPOP's high porosityallows for efficient Zn2+ infiltration through the poresduring charging-discharging cycles and contributes to the efficientutilization of redox-active quinone units. It delivers a specificcapacity of 120 mAh g(-1) at a current density of0.1 A g(-1) with a flat and long discharge plateau,which is critically important to provide a stable voltage output.It provides ultralong cycle life at a current density of 1.0 A g(-1) for 1000 and at 2.0 A g(-1) for 30 000cycles, with initial capacity retention of 95 and 66%, respectively.The co-insertion (Zn2+ and H+) charge storagemechanism was investigated using various electrochemical measurementsand ex/in situ structural characterization techniques, and is explainedherein. These findings contribute to a better understanding of thestructure-property relationship for rPOP and open a new avenuefor new organic cathode materials for high-performance next-generationaqueous batteries.</p></subfield> </datafield> </record>
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