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Isci, Recep; Wan, Li; Topal, Sebahat; Gunturkun, Dilara; Campbell, Alasdair James; Ozturk, Turan
<?xml version='1.0' encoding='utf-8'?> <oai_dc:dc xmlns:dc="http://purl.org/dc/elements/1.1/" xmlns:oai_dc="http://www.openarchives.org/OAI/2.0/oai_dc/" xmlns:xsi="http://www.w3.org/2001/XMLSchema-instance" xsi:schemaLocation="http://www.openarchives.org/OAI/2.0/oai_dc/ http://www.openarchives.org/OAI/2.0/oai_dc.xsd"> <dc:creator>Isci, Recep</dc:creator> <dc:creator>Wan, Li</dc:creator> <dc:creator>Topal, Sebahat</dc:creator> <dc:creator>Gunturkun, Dilara</dc:creator> <dc:creator>Campbell, Alasdair James</dc:creator> <dc:creator>Ozturk, Turan</dc:creator> <dc:date>2022-01-01</dc:date> <dc:description>Two novel donor-pi-acceptor (D-pi-A)-type pull-push materials, M1 and M2, having triphenylamine as a donor and dimesitylboron as an acceptor, linked through a thieno[3,2-b]thiophene (TT) pi-conjugated spacer bearing different functional substituents, such as -PhCN and -Ph, were synthesized and fabricated via a solution process for OLED applications. They exhibited mega Stokes shifts of 120 nm and emissions both in the solid-state and in solution. The monomers M1 and M2 had strong intramolecular charge-transfer behaviors; the solid-state quantum yields were recorded to be 76 and 72% and the solution quantum efficiencies were determined to be 100 and 95%, respectively. The solution-processed OLEDs were fabricated using low turn-on voltages, which had performances with maximum power, current and external quantum efficiencies of around 8 lm W-1, 14.1 cd A(-1) and 4.78%, respectively, displaying emission colors from blue to green and yellowish green. The materials had strong fluorescence emission colors between yellowish and bluish under UV irradiation.</dc:description> <dc:identifier>https://aperta.ulakbim.gov.trrecord/252603</dc:identifier> <dc:identifier>oai:aperta.ulakbim.gov.tr:252603</dc:identifier> <dc:rights>info:eu-repo/semantics/openAccess</dc:rights> <dc:rights>http://www.opendefinition.org/licenses/cc-by</dc:rights> <dc:source>JOURNAL OF MATERIALS CHEMISTRY C 10(29) 10719-10727</dc:source> <dc:title>Solution-processable donor-pi-acceptor type thieno[3,2-b]thiophene derivatives; synthesis, photophysical properties and applications</dc:title> <dc:type>info:eu-repo/semantics/article</dc:type> <dc:type>publication-article</dc:type> </oai_dc:dc>
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