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Modification and Dynamics inside Diamond by Femtosecond Laser Double-Pulse Irradiation

Sakakura, Masaaki; Okada, Takuro; Bharadwaj, Vibhav; Sotillo, Belen; Eaton, Shane M.; Ramponi, Roberta; Serpenguzel, Ali; Gokay, Ulas S.; Shimotsuma, Yasuhiko; Miura, Kiyotaka


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        "affiliation": "Kyoto Univ, Grad Sch Engn, Dept Chem Mat, Kyoto, Japan", 
        "name": "Okada, Takuro"
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      {
        "name": "Bharadwaj, Vibhav"
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      {
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      {
        "name": "Eaton, Shane M."
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      {
        "name": "Ramponi, Roberta"
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      {
        "affiliation": "Koc Univ, Dept Phys, Microphoton Res Lab, Istanbul, Turkey", 
        "name": "Serpenguzel, Ali"
      }, 
      {
        "affiliation": "Koc Univ, Dept Phys, Microphoton Res Lab, Istanbul, Turkey", 
        "name": "Gokay, Ulas S."
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        "affiliation": "Kyoto Univ, Grad Sch Engn, Dept Chem Mat, Kyoto, Japan", 
        "name": "Shimotsuma, Yasuhiko"
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        "affiliation": "Kyoto Univ, Grad Sch Engn, Dept Chem Mat, Kyoto, Japan", 
        "name": "Miura, Kiyotaka"
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    "description": "We investigated modifications and the temporal evolution of the morphology in the photoexcited region inside diamond single crystal after photoexcitation by tightly focused fs laser pulses. We found that double-pulse irradiation with 200-400 fs laser pulses was able to induce a permanent modification in the photoexcited region, while single-pulse irradiation with 100-300 fs laser pulses was not. The modification by double-pulse irradiation became larger for a longer time-difference between the two pulses in the range from 1 ps to 10 ps. The morphology change observed by a pump-probe optical microscope showed that the photoexcited region by double-pulse irradiation was smaller than by single-pulse irradiation, even for the same total pulse energy, with the amplitudes of the laser induced-stress waves being the same. This observation suggests that the photoinduced plasmas by double-pulse irradiation was localized in a smaller region than that by single-pulse irradiation, and the difference in plasma distribution could be the origin of the permanent modification.", 
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Sakakura, M., Okada, T., Bharadwaj, V., Sotillo, B., Eaton, S. M., Ramponi, R., … Miura, K. (2016). Modification and Dynamics inside Diamond by Femtosecond Laser Double-Pulse Irradiation. JOURNAL OF LASER MICRO NANOENGINEERING, 11(3), 346–351. doi:10.2961/jlmn.2016.03.0012

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