Dergi makalesi Açık Erişim
Celebi, Nuray; Soysal, Furkan; Salimi, Kouroush
<?xml version='1.0' encoding='UTF-8'?> <record xmlns="http://www.loc.gov/MARC21/slim"> <leader>00000nam##2200000uu#4500</leader> <datafield tag="245" ind1=" " ind2=" "> <subfield code="a">Spherical shape-defined hollow UiO-66 metal-organic frameworks with superior incident photon scattering for enhanced photoelectrochemical H-2 evolution</subfield> </datafield> <datafield tag="909" ind1="C" ind2="4"> <subfield code="p">JOURNAL OF COLLOID AND INTERFACE SCIENCE</subfield> <subfield code="v">608</subfield> <subfield code="c">1238-1246</subfield> </datafield> <controlfield tag="001">235810</controlfield> <datafield tag="980" ind1=" " ind2=" "> <subfield code="a">user-tubitak-destekli-proje-yayinlari</subfield> </datafield> <datafield tag="520" ind1=" " ind2=" "> <subfield code="a">Herein, spherical hollow N-doped carbon-incorporated UiO-66 metal-organic frameworks (MOF, H-UiO-66) are synthesized using bio-inspired polydopamine (pDA) nanoparticles as multifunctional starting templates. The calculated band properties (E-CB = -0.45 eV and E-VB = 2.05 eV versus normal hydrogen electrode (NHE)) strongly reveals the visible light absorption of H-UiO-66 nanostructures thanks to the spherical shape-defined morphology as well as cavity of the hollow structure. The evaluation of photo-electrochemical (PEC) water splitting performance of H-UiO-66 photoanodes shows maximum photocurrent density as 10.95 mA/cm(2) at 1.53 V versus RHE under LED illumination in which almost no response is recorded at dark. Furthermore, the improved visible-light sensitive PEC water splitting performance of H-UiO-66 photoanodes could be attributed to the main advantages of the one-pot synthesis method of hollow MOFs using multifunctional pDA as follows: i) the hollow morphology provides superior incident photon scattering and multi-reflection of photons inside the MOF cavity; ii) presence of N-doped carbon incorporated morphology facilitates the absorption of water molecules as well as the pi-polar interaction between water and carbon; and iii) the reduced bang-gap led to the optical localization of light within HUiO-66 clusters, suggesting a new generation of heterogeneous well-defined nanostructures for sustainable PEC hydrogen production. (C) 2021 Elsevier Inc. All rights reserved.</subfield> </datafield> <datafield tag="650" ind1="1" ind2="7"> <subfield code="2">opendefinition.org</subfield> <subfield code="a">cc-by</subfield> </datafield> <datafield tag="700" ind1=" " ind2=" "> <subfield code="u">Ankara Yildirim Beyazit Univ, Fac Engn & Nat Sci, Dept Chem Engn, TR-06010 Ankara, Turkey</subfield> <subfield code="a">Soysal, Furkan</subfield> </datafield> <datafield tag="700" ind1=" " ind2=" "> <subfield code="u">Ankara Yildirim Beyazit Univ, Fac Engn & Nat Sci, Dept Chem Engn, TR-06010 Ankara, Turkey</subfield> <subfield code="a">Salimi, Kouroush</subfield> </datafield> <datafield tag="980" ind1=" " ind2=" "> <subfield code="b">article</subfield> <subfield code="a">publication</subfield> </datafield> <datafield tag="542" ind1=" " ind2=" "> <subfield code="l">open</subfield> </datafield> <datafield tag="100" ind1=" " ind2=" "> <subfield code="u">Ankara Yildirim Beyazit Univ, Fac Engn & Nat Sci, Dept Energy Syst Engn, TR-06010 Ankara, Turkey</subfield> <subfield code="a">Celebi, Nuray</subfield> </datafield> <datafield tag="260" ind1=" " ind2=" "> <subfield code="c">2022-01-01</subfield> </datafield> <controlfield tag="005">20221007092954.0</controlfield> <datafield tag="909" ind1="C" ind2="O"> <subfield code="o">oai:aperta.ulakbim.gov.tr:235810</subfield> <subfield code="p">user-tubitak-destekli-proje-yayinlari</subfield> </datafield> <datafield tag="856" ind1="4" ind2=" "> <subfield code="z">md5:240edd053e0c2226caee433c93e12074</subfield> <subfield code="s">260</subfield> <subfield code="u">https://aperta.ulakbim.gov.trrecord/235810/files/bib-69465c82-8a63-46fa-9781-fd024b9a6cf5.txt</subfield> </datafield> <datafield tag="540" ind1=" " ind2=" "> <subfield code="u">http://www.opendefinition.org/licenses/cc-by</subfield> <subfield code="a">Creative Commons Attribution</subfield> </datafield> <datafield tag="024" ind1=" " ind2=" "> <subfield code="a">10.1016/j.jcis.2021.10.145</subfield> <subfield code="2">doi</subfield> </datafield> </record>
Görüntülenme | 19 |
İndirme | 4 |
Veri hacmi | 1.0 kB |
Tekil görüntülenme | 19 |
Tekil indirme | 4 |